TY - JOUR
T1 - Copper-Free Click Enabled Triazabutadiene for Bioorthogonal Protein Functionalization
AU - Wijetunge, Anjalee N.
AU - Davis, Garrett J.
AU - Shadmehr, Mehrdad
AU - Townsend, Julia A.
AU - Marty, Michael T.
AU - Jewett, John C.
N1 - Funding Information: This work was supported in part by the NSF-CAREER award, given to J.C.J. (CHE-1552568). Additional funding to J.A.T. and M.T.M. was provided by the National Institute of General Medical Sciences and National Institutes of Health (T32 GM008804 to J.A.T. and R35 GM128624 to M.T.M.). All NMR data were collected in the NMR facility at the University of Arizona. The purchase of the Bruker AVANCE III 400 MHz spectrometer was supported by NSF grant 840336 and the University of Arizona. The purchase and upgrade of the Bruker AVANCE DRX 500 MHz spectrometer was partially supported by NSF grant 9214383, the Office of Naval Research, and the University of Arizona. The purchase of the Bruker NEO 500 MHz spectrometer was supported by NSF grant 1920234 and the University of Arizona. All FTIR spectra were collected in the W.M. Keck Center for Nano-Scale Imaging in the Department of Chemistry and Biochemistry at the University of Arizona. This instrument purchase was supported by Arizona Technology and Research Initiative Fund (A.R.S.§15-1648). We thank Kristen Keck and Yelena Feinstein at the University of Arizona Analytical & Biological Mass Spectrometry Facility for help with the MS analysis. Publisher Copyright: © 2021 American Chemical Society.
PY - 2021/2/17
Y1 - 2021/2/17
N2 - Aryl diazonium ions have long been used in bioconjugation due to their reactivity toward electron-rich aryl residues, such as tyrosine. However, their utility in biological systems has been restricted due to the requirement of harsh conditions for their generation in situ, as well as limited hydrolytic stability. Previous work describing a scaffold known as triazabutadiene (TBD) has shown the ability to protect aryl diazonium ions allowing for increased synthetic utility, as well as triggered release under biologically relevant conditions. Herein, we describe the synthesis and application of a novel TBD, capable of installation of a cyclooctyne on protein surfaces for later use of copper-free click reactions involving functional azides. The probe shows efficient protein labeling across a wide pH range that can be accomplished in a convenient and timely manner. Orthogonality of the cyclooctyne modification was showcased by labeling a model protein in the presence of hen egg proteins, using an azide-containing fluorophore. We further confirmed that the azobenzene modification can be cleaved using sodium dithionite treatment.
AB - Aryl diazonium ions have long been used in bioconjugation due to their reactivity toward electron-rich aryl residues, such as tyrosine. However, their utility in biological systems has been restricted due to the requirement of harsh conditions for their generation in situ, as well as limited hydrolytic stability. Previous work describing a scaffold known as triazabutadiene (TBD) has shown the ability to protect aryl diazonium ions allowing for increased synthetic utility, as well as triggered release under biologically relevant conditions. Herein, we describe the synthesis and application of a novel TBD, capable of installation of a cyclooctyne on protein surfaces for later use of copper-free click reactions involving functional azides. The probe shows efficient protein labeling across a wide pH range that can be accomplished in a convenient and timely manner. Orthogonality of the cyclooctyne modification was showcased by labeling a model protein in the presence of hen egg proteins, using an azide-containing fluorophore. We further confirmed that the azobenzene modification can be cleaved using sodium dithionite treatment.
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U2 - 10.1021/acs.bioconjchem.0c00677
DO - 10.1021/acs.bioconjchem.0c00677
M3 - Article
C2 - 33492934
SN - 1043-1802
VL - 32
SP - 254
EP - 258
JO - Bioconjugate chemistry
JF - Bioconjugate chemistry
IS - 2
ER -