Cross-relaxation energy transfer in Tm 3+ doped tellurite glass

Jianfeng Wu; Shibin Jiang; Tiequn Qiu; Michael Morrell; Axel Schulzgen; Nasser Peyghambarian

doi:10.1117/12.592289

Cross-relaxation energy transfer in Tm ³⁺ doped tellurite glass

Jianfeng Wu, Shibin Jiang, Tiequn Qiu, Michael Morrell, Axel Schulzgen, Nasser Peyghambarian

Research output: Contribution to journal › Conference article › peer-review

9 Scopus citations

Abstract

A self-calibrating fluorescence spectroscopy technique was applied to study cross-relaxation ³H ₄, ³H ₆ → ³F ₄, ³F ₄, and energy migration ³H ₄, ³H ₆ → ³F ₄, ³F ₄, of the Tm ³⁺ Ions doped in the tellurite glass. These glasses are investigated for their use in realization of 2 micron fiber lasers. Micro and macro-parameters of the energy transfer and migration were calculated by the means of the model of phonon-assistant multi-polar interaction and hoping mode. Steady rate equation analysis was used to fit the experimental fluorescence ratio of samples with different concentrations. We found that high-order (dipole-quadrupole) interaction was the dominant mechanism in the energy transfer of Thulium ions.

Original language	English (US)
Article number	23
Pages (from-to)	152-161
Number of pages	10
Journal	Proceedings of SPIE - The International Society for Optical Engineering
Volume	5723
DOIs	https://doi.org/10.1117/12.592289
State	Published - 2005
Event	Optical Components and Materials II - San Jose, CA, United States Duration: Jan 24 2005 → Jan 25 2005

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Computer Science Applications
Applied Mathematics
Electrical and Electronic Engineering

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10.1117/12.592289

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title = "Cross-relaxation energy transfer in Tm 3+ doped tellurite glass",

abstract = "A self-calibrating fluorescence spectroscopy technique was applied to study cross-relaxation 3H 4, 3H 6 → 3F 4, 3F 4, and energy migration 3H 4, 3H 6 → 3F 4, 3F 4, of the Tm 3+ Ions doped in the tellurite glass. These glasses are investigated for their use in realization of 2 micron fiber lasers. Micro and macro-parameters of the energy transfer and migration were calculated by the means of the model of phonon-assistant multi-polar interaction and hoping mode. Steady rate equation analysis was used to fit the experimental fluorescence ratio of samples with different concentrations. We found that high-order (dipole-quadrupole) interaction was the dominant mechanism in the energy transfer of Thulium ions.",

author = "Jianfeng Wu and Shibin Jiang and Tiequn Qiu and Michael Morrell and Axel Schulzgen and Nasser Peyghambarian",

year = "2005",

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pages = "152--161",

journal = "Proceedings of SPIE - The International Society for Optical Engineering",

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note = "Optical Components and Materials II ; Conference date: 24-01-2005 Through 25-01-2005",

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T1 - Cross-relaxation energy transfer in Tm 3+ doped tellurite glass

AU - Wu, Jianfeng

AU - Jiang, Shibin

AU - Qiu, Tiequn

AU - Morrell, Michael

AU - Schulzgen, Axel

AU - Peyghambarian, Nasser

PY - 2005

Y1 - 2005

N2 - A self-calibrating fluorescence spectroscopy technique was applied to study cross-relaxation 3H 4, 3H 6 → 3F 4, 3F 4, and energy migration 3H 4, 3H 6 → 3F 4, 3F 4, of the Tm 3+ Ions doped in the tellurite glass. These glasses are investigated for their use in realization of 2 micron fiber lasers. Micro and macro-parameters of the energy transfer and migration were calculated by the means of the model of phonon-assistant multi-polar interaction and hoping mode. Steady rate equation analysis was used to fit the experimental fluorescence ratio of samples with different concentrations. We found that high-order (dipole-quadrupole) interaction was the dominant mechanism in the energy transfer of Thulium ions.

AB - A self-calibrating fluorescence spectroscopy technique was applied to study cross-relaxation 3H 4, 3H 6 → 3F 4, 3F 4, and energy migration 3H 4, 3H 6 → 3F 4, 3F 4, of the Tm 3+ Ions doped in the tellurite glass. These glasses are investigated for their use in realization of 2 micron fiber lasers. Micro and macro-parameters of the energy transfer and migration were calculated by the means of the model of phonon-assistant multi-polar interaction and hoping mode. Steady rate equation analysis was used to fit the experimental fluorescence ratio of samples with different concentrations. We found that high-order (dipole-quadrupole) interaction was the dominant mechanism in the energy transfer of Thulium ions.

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EP - 161

JO - Proceedings of SPIE - The International Society for Optical Engineering

JF - Proceedings of SPIE - The International Society for Optical Engineering

M1 - 23

T2 - Optical Components and Materials II

Y2 - 24 January 2005 through 25 January 2005

ER -

Cross-relaxation energy transfer in Tm ³⁺ doped tellurite glass

Abstract

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