TY - JOUR
T1 - Lensfree Air-Quality Monitoring of Fine and Ultrafine Particulate Matter Using Vapor-Condensed Nanolenses
AU - Baker, Maryam
AU - Gollier, Florian
AU - Melzer, Jeffrey E.
AU - McLeod, Euan
N1 - Funding Information: This research was supported by a University of Arizona Building a Changing World Restruct Seed Grant and a University of Arizona Water, Environmental, and Energy Solutions TRIF Equipment Grant. The authors acknowledge NASA grants #NNX12AL47G and #NNX15AJ22G and NSF grant #1531243 for funding of the instrumentation in the Kuiper Materials Imaging and Characterization Facility at the University of Arizona. This work was performed in part at the Micro/Nano Fabrication Center at the University of Arizona. The authors would like to acknowledge Dr. Mary Kay O’Rourke and her students Emmanuel Gonzalez-Figueroa and Muath Almoslem for sharing access to the Children’s Park. The authors would like to acknowledge Mike Draper for the continued access to the Pima County Air-Quality Monitoring site at the Children’s Park and for answering their questions about the air-quality monitoring equipment on site. Publisher Copyright: © 2023 American Chemical Society.
PY - 2023/7/14
Y1 - 2023/7/14
N2 - Current commercial air-quality monitoring devices lack a large dynamic range, especially at the small, ultrafine size scale. Furthermore, there is a low density of air-quality monitoring stations, reducing the precision with which local particulate matter hazards can be tracked. Here, we show a low-cost, lensfree, and portable air-quality monitoring device (LPAQD) that can detect and measure micron-sized particles down to 100 nm-sized particles, with the capability to track and measure particles in real time throughout a day and the ability to accurately measure particulate matter densities as low as 3 μg m-3. A vapor-condensed film is deposited onto the coverslip used to collect particles before the LPAQD is deployed at outdoor monitoring sites. The vapor-condensed film increases the scattering cross section of particles smaller than the pixel size, enabling the sub-pixel and sub-diffraction-limit-sized particles to be detected. The high dynamic range, low cost, and portability of this device can enable citizens to monitor their own air quality to hopefully impact user decisions that reduce the risk for particulate matter-related diseases.
AB - Current commercial air-quality monitoring devices lack a large dynamic range, especially at the small, ultrafine size scale. Furthermore, there is a low density of air-quality monitoring stations, reducing the precision with which local particulate matter hazards can be tracked. Here, we show a low-cost, lensfree, and portable air-quality monitoring device (LPAQD) that can detect and measure micron-sized particles down to 100 nm-sized particles, with the capability to track and measure particles in real time throughout a day and the ability to accurately measure particulate matter densities as low as 3 μg m-3. A vapor-condensed film is deposited onto the coverslip used to collect particles before the LPAQD is deployed at outdoor monitoring sites. The vapor-condensed film increases the scattering cross section of particles smaller than the pixel size, enabling the sub-pixel and sub-diffraction-limit-sized particles to be detected. The high dynamic range, low cost, and portability of this device can enable citizens to monitor their own air quality to hopefully impact user decisions that reduce the risk for particulate matter-related diseases.
KW - air-quality monitoring
KW - digital holography
KW - lensfree microscopy
KW - nanolenses
KW - ultrafines
KW - vapor-condensed film
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U2 - 10.1021/acsanm.3c01154
DO - 10.1021/acsanm.3c01154
M3 - Article
SN - 2574-0970
VL - 6
SP - 11166
EP - 11174
JO - ACS Applied Nano Materials
JF - ACS Applied Nano Materials
IS - 13
ER -