Abstract
Time-dependent simulations of the single and double ionization of atomic Calcium using a two-active-electron model were performed. These simulations were implemented within a basis set representation, allowing for an unambiguous calculation of the single- and double-ionization probabilities. Thus, the electron wave packet dynamics have revealed the main feature responsible for the enhancement of double ionization which was observed in a recent adaptive control experiment. The simulations show that the initial part of the pulse prepares a coherent superposition of excited states above the first ionization threshold.
Original language | English (US) |
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Article number | 053407 |
Pages (from-to) | 053407/1-053407/9 |
Journal | Physical Review A - Atomic, Molecular, and Optical Physics |
Volume | 66 |
Issue number | 5 |
State | Published - Nov 2002 |
Externally published | Yes |
ASJC Scopus subject areas
- Atomic and Molecular Physics, and Optics