Tracking of oxide formation in laser-produced uranium plasmas

P. J. Skrodzki; M. Burger; I. Jovanovic; M. C. Phillips; B. E. Brumfield; S. S. Harilal

doi:10.1364/OL.43.005118

Tracking of oxide formation in laser-produced uranium plasmas

P. J. Skrodzki, M. Burger, I. Jovanovic, M. C. Phillips, B. E. Brumfield, S. S. Harilal

Research output: Contribution to journal › Article › peer-review

27 Scopus citations

Abstract

We use a spatially and temporally resolved emission tracking technique based on optical emission spectroscopy to map the evolution of emission features from uranium and its compounds in a plasma produced by a nanosecond laser. We observe quenching of the emission from neutral uranium (591.538 nm) and uranium monoxide (593.55 nm) species with increasing oxygen concentration and discuss possible reaction pathways for dissociation or formation of higher uranium oxides (U_xO_y).We further identify spectral features between 320 nm and 380 nm and between 520 nm and 640 nm, which we attribute to UxOy .

Original language	English (US)
Pages (from-to)	5118-5121
Number of pages	4
Journal	Optics letters
Volume	43
Issue number	20
DOIs	https://doi.org/10.1364/OL.43.005118
State	Published - Oct 15 2018
Externally published	Yes

ASJC Scopus subject areas

Atomic and Molecular Physics, and Optics

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title = "Tracking of oxide formation in laser-produced uranium plasmas",

abstract = "We use a spatially and temporally resolved emission tracking technique based on optical emission spectroscopy to map the evolution of emission features from uranium and its compounds in a plasma produced by a nanosecond laser. We observe quenching of the emission from neutral uranium (591.538 nm) and uranium monoxide (593.55 nm) species with increasing oxygen concentration and discuss possible reaction pathways for dissociation or formation of higher uranium oxides (UxOy).We further identify spectral features between 320 nm and 380 nm and between 520 nm and 640 nm, which we attribute to UxOy .",

author = "Skrodzki, {P. J.} and M. Burger and I. Jovanovic and Phillips, {M. C.} and Brumfield, {B. E.} and Harilal, {S. S.}",

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AU - Skrodzki, P. J.

AU - Burger, M.

AU - Jovanovic, I.

AU - Phillips, M. C.

AU - Brumfield, B. E.

AU - Harilal, S. S.

PY - 2018/10/15

Y1 - 2018/10/15

N2 - We use a spatially and temporally resolved emission tracking technique based on optical emission spectroscopy to map the evolution of emission features from uranium and its compounds in a plasma produced by a nanosecond laser. We observe quenching of the emission from neutral uranium (591.538 nm) and uranium monoxide (593.55 nm) species with increasing oxygen concentration and discuss possible reaction pathways for dissociation or formation of higher uranium oxides (UxOy).We further identify spectral features between 320 nm and 380 nm and between 520 nm and 640 nm, which we attribute to UxOy .

AB - We use a spatially and temporally resolved emission tracking technique based on optical emission spectroscopy to map the evolution of emission features from uranium and its compounds in a plasma produced by a nanosecond laser. We observe quenching of the emission from neutral uranium (591.538 nm) and uranium monoxide (593.55 nm) species with increasing oxygen concentration and discuss possible reaction pathways for dissociation or formation of higher uranium oxides (UxOy).We further identify spectral features between 320 nm and 380 nm and between 520 nm and 640 nm, which we attribute to UxOy .

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Tracking of oxide formation in laser-produced uranium plasmas

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